Literature DB >> 18763923

Minimal model for kinetic arrest.

P Pal1, C S O'Hern, J Blawzdziewicz, E R Dufresne, R Stinchcombe.   

Abstract

To elucidate slow dynamics in glassy materials, we introduce the figure-8 model in which N hard blocks undergo Brownian motion around a circuit in the shape of a figure 8. This system undergoes kinetic arrest at a critical packing fraction phi=phi g<1 , and for phi approximately phi g long-time diffusion is controlled by rare, cooperative, "junction-crossing" particle rearrangements. We find that the average time between junction crossings tau JC, and hence the structural relaxation time, does not simply scale with the configurational volume Omega c of transition states, because tau JC also depends on the time to complete a junction crossing. The importance of these results in understanding cage-breaking dynamics in glassy systems is discussed.

Entities:  

Year:  2008        PMID: 18763923     DOI: 10.1103/PhysRevE.78.011111

Source DB:  PubMed          Journal:  Phys Rev E Stat Nonlin Soft Matter Phys        ISSN: 1539-3755


  2 in total

1.  Cooperative strings and glassy interfaces.

Authors:  Thomas Salez; Justin Salez; Kari Dalnoki-Veress; Elie Raphaël; James A Forrest
Journal:  Proc Natl Acad Sci U S A       Date:  2015-06-22       Impact factor: 11.205

2.  Collective Motion of Repulsive Brownian Particles in Single-File Diffusion with and without Overtaking.

Authors:  Takeshi Ooshida; Susumu Goto; Michio Otsuki
Journal:  Entropy (Basel)       Date:  2018-08-02       Impact factor: 2.524

  2 in total

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