Literature DB >> 18648436

Antenna-mediated back-scattering efficiency in infrared near-field microscopy.

M Brehm1, A Schliesser, F Cajko, I Tsukerman, F Keilmann.   

Abstract

We evaluate the efficiency of back-scattering, eta(B), from a standard cantilevered AFM probe contacting a flat sample, and also the back-scattering phase. Both quantities are spectroscopically determined over a broad 9-12 mum wavelength range by coherent frequency-comb Fourier-transform spectroscopy (c-FTIR). While Fresnel reflectivity contributes a key factor with the SiC Reststrahlen edge at 975 cm(-1)as previously documented, we observe spectral effects ascribable to antenna resonances involving the shaft, cantilever, and sample. Most conspicuous is strong (eta(B) = 13%), resonant back-scattering at 955 cm(-1), a frequency that suggests the involvement of surface-phonon-polariton excitation, when the tip probes the area near a SiC/Au boundary. The probe's antenna properties are elucidated by numerically simulating the near fields, the fields in the radiation zone, and the far-field scattering distributions. The simulations are performed for a realistic tip/sample configuration with a three-orders-of-magnitude scale variation. The results suggest a standing-surface-plasmon-polariton pattern along the shaft, as well as far-field antenna lobes that change with the sample's dielectric properties.

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Year:  2008        PMID: 18648436     DOI: 10.1364/oe.16.011203

Source DB:  PubMed          Journal:  Opt Express        ISSN: 1094-4087            Impact factor:   3.894


  4 in total

1.  Infrared-spectroscopic nanoimaging with a thermal source.

Authors:  F Huth; M Schnell; J Wittborn; N Ocelic; R Hillenbrand
Journal:  Nat Mater       Date:  2011-04-17       Impact factor: 43.841

2.  Closed-loop atomic force microscopy-infrared spectroscopic imaging for nanoscale molecular characterization.

Authors:  Seth Kenkel; Shachi Mittal; Rohit Bhargava
Journal:  Nat Commun       Date:  2020-06-26       Impact factor: 14.919

3.  Infrared-spectroscopic, dynamic near-field microscopy of living cells and nanoparticles in water.

Authors:  Korbinian J Kaltenecker; Thorsten Gölz; Enrico Bau; Fritz Keilmann
Journal:  Sci Rep       Date:  2021-11-08       Impact factor: 4.379

4.  Correlative infrared-electron nanoscopy reveals the local structure-conductivity relationship in zinc oxide nanowires.

Authors:  J M Stiegler; R Tena-Zaera; O Idigoras; A Chuvilin; R Hillenbrand
Journal:  Nat Commun       Date:  2012       Impact factor: 14.919

  4 in total

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