Literature DB >> 18518104

Adiabatic approximation in nonperturbative time-dependent density-functional theory.

M Thiele1, E K U Gross, S Kümmel.   

Abstract

We construct the exact exchange-correlation potential of time-dependent density-functional theory and the approximation to it that is adiabatic but exact otherwise. For the strong-field double ionization of the Helium atom these two potentials are virtually identical. Thus, memory effects play a negligible role in this paradigm process of nonlinear, nonperturbative electron dynamics. We identify the regime of high-frequency excitations where the adiabatic approximation breaks down and explicitly calculate the nonadiabatic contribution to the exchange-correlation potential.

Entities:  

Year:  2008        PMID: 18518104     DOI: 10.1103/PhysRevLett.100.153004

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  4 in total

1.  Time-resolved spectroscopy in time-dependent density functional theory: an exact condition.

Authors:  Johanna I Fuks; Kai Luo; Ernesto D Sandoval; Neepa T Maitra
Journal:  Phys Rev Lett       Date:  2015-05-05       Impact factor: 9.161

2.  Kinetic and interaction components of the exact time-dependent correlation potential.

Authors:  Kai Luo; Johanna I Fuks; Ernesto D Sandoval; Peter Elliott; Neepa T Maitra
Journal:  J Chem Phys       Date:  2014-05-14       Impact factor: 3.488

Review 3.  Carbon Nanodots from an In Silico Perspective.

Authors:  Francesca Mocci; Leon de Villiers Engelbrecht; Chiara Olla; Antonio Cappai; Maria Francesca Casula; Claudio Melis; Luigi Stagi; Aatto Laaksonen; Carlo Maria Carbonaro
Journal:  Chem Rev       Date:  2022-08-10       Impact factor: 72.087

4.  Superadiabatic Forces via the Acceleration Gradient in Quantum Many-Body Dynamics.

Authors:  Moritz Brütting; Thomas Trepl; Daniel de Las Heras; Matthias Schmidt
Journal:  Molecules       Date:  2019-10-11       Impact factor: 4.411

  4 in total

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