Literature DB >> 17764338

Data acquisition schemes for continuous two-particle time-of-flight coincidence experiments.

Andras Bodi1, Bálint Sztáray, Tomas Baer, Melanie Johnson, Thomas Gerber.   

Abstract

Three data acquisition schemes for two-particle coincidence experiments with a continuous source are discussed. The single-start/single-stop technique, implemented with a time-to-pulse-height converter, results in a complicated spectrum and breaks down severely at high count rates. The single-start/multiple-stop setup, based on a time-to-digital converter and the first choice in today's similar coincidence experiments, performs significantly better at high count rates, but its performance is still hampered if the time-of-flight range is large, and the false coincidence background is variable if the event frequency and the collection efficiency of the starts are both high. A straightforward, multistart/multistop setup is proposed for coincidence experiments. By collecting all detector data, it ensures the highest signal-to-noise ratio, constant background, and fast data acquisition and can now be easily constructed with commercially available time-to-digital converters. Analytical and numerically evaluated formulas are derived to characterize the performance of each setup in a variety of environments. Computer simulated spectra are presented to illustrate the analytically predicted features of the various raw time-of-flight distributions obtained with each technique.

Mesh:

Year:  2007        PMID: 17764338     DOI: 10.1063/1.2776012

Source DB:  PubMed          Journal:  Rev Sci Instrum        ISSN: 0034-6748            Impact factor:   1.523


  6 in total

1.  Elucidation of radical- and oxygenate-driven paths in zeolite-catalysed conversion of methanol and methyl chloride to hydrocarbons.

Authors:  Alessia Cesarini; Sharon Mitchell; Guido Zichittella; Mikhail Agrachev; Stefan P Schmid; Gunnar Jeschke; Zeyou Pan; Andras Bodi; Patrick Hemberger; Javier Pérez-Ramírez
Journal:  Nat Catal       Date:  2022-06-27

2.  Understanding the mechanism of catalytic fast pyrolysis by unveiling reactive intermediates in heterogeneous catalysis.

Authors:  Patrick Hemberger; Victoria B F Custodis; Andras Bodi; Thomas Gerber; Jeroen A van Bokhoven
Journal:  Nat Commun       Date:  2017-06-29       Impact factor: 14.919

3.  On the absolute photoionization cross section and threshold photoelectron spectrum of two reactive ketenes in lignin valorization: fulvenone and 2-carbonyl cyclohexadienone.

Authors:  Zeyou Pan; Andras Bodi; Jeroen A van Bokhoven; Patrick Hemberger
Journal:  Phys Chem Chem Phys       Date:  2022-02-09       Impact factor: 3.676

4.  Unimolecular reaction energies for polycyclic aromatic hydrocarbon ions.

Authors:  Brandi West; Sarah Rodriguez Castillo; Alicia Sit; Sabria Mohamad; Bethany Lowe; Christine Joblin; Andras Bodi; Paul M Mayer
Journal:  Phys Chem Chem Phys       Date:  2018-03-07       Impact factor: 3.676

5.  Photoionisation of the tropyl radical.

Authors:  Kathrin H Fischer; Patrick Hemberger; Andras Bodi; Ingo Fischer
Journal:  Beilstein J Org Chem       Date:  2013-04-09       Impact factor: 2.883

6.  Threshold Photoelectron Spectroscopy of IO and HOI.

Authors:  Domenik Schleier; Engelbert Reusch; Lisa Lummel; Patrick Hemberger; Ingo Fischer
Journal:  Chemphyschem       Date:  2019-09-11       Impact factor: 3.102

  6 in total

北京卡尤迪生物科技股份有限公司 © 2022-2023.