Literature DB >> 17508808

Spontaneous and induced dynamic correlations in glass formers. II. Model calculations and comparison to numerical simulations.

L Berthier1, G Biroli, J-P Bouchaud, W Kob, K Miyazaki, D R Reichman.   

Abstract

We study in detail the predictions of various theoretical approaches, in particular, mode-coupling theory (MCT) and kinetically constrained models (KCMs), concerning the time, temperature, and wave vector dependence of multipoint correlation functions that quantify the strength of both induced and spontaneous dynamical fluctuations. We also discuss the precise predictions of MCT concerning the statistical ensemble and microscopic dynamics dependence of these multipoint correlation functions. These predictions are compared to simulations of model fragile and strong glass-forming liquids. Overall, MCT fares quite well in the fragile case, in particular, explaining the observed crucial role of the statistical ensemble and microscopic dynamics, while MCT predictions do not seem to hold in the strong case. KCMs provide a simplified framework for understanding how these multipoint correlation functions may encode dynamic correlations in glassy materials. However, our analysis highlights important unresolved questions concerning the application of KCMs to supercooled liquids.

Entities:  

Year:  2007        PMID: 17508808     DOI: 10.1063/1.2721555

Source DB:  PubMed          Journal:  J Chem Phys        ISSN: 0021-9606            Impact factor:   3.488


  8 in total

1.  Dynamic and thermodynamic crossover scenarios in the Kob-Andersen mixture: Insights from multi-CPU and multi-GPU simulations.

Authors:  Daniele Coslovich; Misaki Ozawa; Walter Kob
Journal:  Eur Phys J E Soft Matter       Date:  2018-05-17       Impact factor: 1.890

2.  Bond orientational order in liquids: Towards a unified description of water-like anomalies, liquid-liquid transition, glass transition, and crystallization: Bond orientational order in liquids.

Authors:  Hajime Tanaka
Journal:  Eur Phys J E Soft Matter       Date:  2012-10-31       Impact factor: 1.890

Review 3.  The Interplay between the Theories of Mode Coupling and of Percolation Transition in Attractive Colloidal Systems.

Authors:  Francesco Mallamace; Giuseppe Mensitieri; Martina Salzano de Luna; Paola Lanzafame; Georgia Papanikolaou; Domenico Mallamace
Journal:  Int J Mol Sci       Date:  2022-05-10       Impact factor: 6.208

4.  MD simulation of concentrated polymer solutions: structural relaxation near the glass transition.

Authors:  S Peter; H Meyer; J Baschnagel
Journal:  Eur Phys J E Soft Matter       Date:  2009-02       Impact factor: 1.890

5.  Quantitative field theory of the glass transition.

Authors:  Silvio Franz; Hugo Jacquin; Giorgio Parisi; Pierfrancesco Urbani; Francesco Zamponi
Journal:  Proc Natl Acad Sci U S A       Date:  2012-10-29       Impact factor: 11.205

6.  Glass-like characteristics of intracellular motion in human cells.

Authors:  Christoffer Åberg; Bert Poolman
Journal:  Biophys J       Date:  2021-04-19       Impact factor: 3.699

7.  Study of dynamical heterogeneities in colloidal nanoclay suspensions approaching dynamical arrest.

Authors:  Paramesh Gadige; Debasish Saha; Sanjay Kumar Behera; Ranjini Bandyopadhyay
Journal:  Sci Rep       Date:  2017-08-14       Impact factor: 4.379

8.  Scaling and universality in glass transition.

Authors:  Antonio de Candia; Annalisa Fierro; Antonio Coniglio
Journal:  Sci Rep       Date:  2016-05-25       Impact factor: 4.379

  8 in total

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