Literature DB >> 17501609

Mosaic multistate scenario versus one-state description of supercooled liquids.

Andrea Cavagna1, Tomás S Grigera, Paolo Verrocchio.   

Abstract

According to the mosaic scenario, relaxation in supercooled liquids is ruled by two competing mechanisms: surface tension, opposing the creation of local excitations, and entropy, providing the drive to the configurational rearrangement of a given region. We test this scenario through numerical simulations well below the Mode Coupling temperature. For an equilibrated configuration, we freeze all the particles outside a sphere and study the thermodynamics of this sphere. The frozen environment acts as a pinning field. Measuring the overlap between the unpinned and pinned equilibrium configurations of the sphere, we can see whether it has switched to a different state. We do not find any clear evidence of the mosaic scenario. Rather, our results seem compatible with the existence of a single (liquid) state. However, we find evidence of a growing static correlation length, apparently unrelated to the mosaic one.

Year:  2007        PMID: 17501609     DOI: 10.1103/PhysRevLett.98.187801

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  2 in total

1.  Testing "microscopic" theories of glass-forming liquids.

Authors:  L Berthier; G Tarjus
Journal:  Eur Phys J E Soft Matter       Date:  2011-09-23       Impact factor: 1.890

2.  The liquid-amorphous phase transition, slow dynamics and dynamical heterogeneity for bulk iron: a molecular dynamics simulation.

Authors:  Kien Huu Pham; Trang Thi Thuy Giap
Journal:  RSC Adv       Date:  2021-10-04       Impact factor: 4.036

  2 in total

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