Literature DB >> 16492746

Depth sectioning with the aberration-corrected scanning transmission electron microscope.

Albina Y Borisevich1, Andrew R Lupini, Stephen J Pennycook.   

Abstract

The ability to correct the aberrations of the probe-forming lens in the scanning transmission electron microscope provides not only a significant improvement in transverse resolution but in addition brings depth resolution at the nanometer scale. Aberration correction therefore opens up the possibility of 3D imaging by optical sectioning. Here we develop a definition for the depth resolution for scanning transmission electron microscope depth sectioning and present initial results from this method. Objects such as catalytic metal clusters and single atoms on various support materials are imaged in three dimensions with a resolution of several nanometers. Effective focal depth is determined by statistical analysis and the contributing factors are discussed. Finally, current challenges and future capabilities available through new instruments are discussed.

Entities:  

Year:  2006        PMID: 16492746      PMCID: PMC1413870          DOI: 10.1073/pnas.0507105103

Source DB:  PubMed          Journal:  Proc Natl Acad Sci U S A        ISSN: 0027-8424            Impact factor:   11.205


  9 in total

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Authors:  P A Midgley; M Weyland
Journal:  Ultramicroscopy       Date:  2003-09       Impact factor: 2.689

2.  HAADF-STEM imaging with sub-angstrom probes: a full Bloch wave analysis.

Authors:  Yiping Peng; Peter D Nellist; Stephen J Pennycook
Journal:  J Electron Microsc (Tokyo)       Date:  2004

3.  Direct sub-angstrom imaging of a crystal lattice.

Authors:  P D Nellist; M F Chisholm; N Dellby; O L Krivanek; M F Murfitt; Z S Szilagyi; A R Lupini; A Borisevich; W H Sides; S J Pennycook
Journal:  Science       Date:  2004-09-17       Impact factor: 47.728

4.  Spectroscopic imaging of single atoms within a bulk solid.

Authors:  M Varela; S D Findlay; A R Lupini; H M Christen; A Y Borisevich; N Dellby; O L Krivanek; P D Nellist; M P Oxley; L J Allen; S J Pennycook
Journal:  Phys Rev Lett       Date:  2004-03-03       Impact factor: 9.161

5.  Visibility of single atoms.

Authors:  A V Crewe; J Wall; J Langmore
Journal:  Science       Date:  1970-06-12       Impact factor: 47.728

6.  Element-selective single atom imaging.

Authors:  K Suenaga; M Tence; C Mory; C Colliex; H Kato; T Okazaki; H Shinohara; K Hirahara; S Bandow; S Iijima
Journal:  Science       Date:  2000-12-22       Impact factor: 47.728

7.  Atomic-scale imaging of individual dopant atoms and clusters in highly n-type bulk Si.

Authors:  P M Voyles; D A Muller; J L Grazul; P H Citrin; H-J L Gossmann
Journal:  Nature       Date:  2002-04-25       Impact factor: 49.962

8.  Towards sub-0.5 A electron beams.

Authors:  O L Krivanek; P D Nellist; N Dellby; M F Murfitt; Z Szilagyi
Journal:  Ultramicroscopy       Date:  2003-09       Impact factor: 2.689

9.  Dopants adsorbed as single atoms prevent degradation of catalysts.

Authors:  Sanwu Wang; Albina Y Borisevich; Sergey N Rashkeev; Michael V Glazoff; Karl Sohlberg; Stephen J Pennycook; Sokrates T Pantelides
Journal:  Nat Mater       Date:  2004-02-22       Impact factor: 43.841

  9 in total
  13 in total

1.  Atomic-scale imaging of individual dopant atoms in a buried interface.

Authors:  N Shibata; S D Findlay; S Azuma; T Mizoguchi; T Yamamoto; Y Ikuhara
Journal:  Nat Mater       Date:  2009-06-21       Impact factor: 43.841

2.  Synthesis, Surface Studies, Composition and Structural Characterization of CdSe, Core/Shell, and Biologically Active Nanocrystals.

Authors:  Sandra J Rosenthal; James McBride; Stephen J Pennycook; Leonard C Feldman
Journal:  Surf Sci Rep       Date:  2007-04-30       Impact factor: 12.267

3.  Tutorial: structural characterization of isolated metal atoms and subnanometric metal clusters in zeolites.

Authors:  Lichen Liu; Miguel Lopez-Haro; Jose J Calvino; Avelino Corma
Journal:  Nat Protoc       Date:  2020-09-04       Impact factor: 13.491

4.  Optimized deconvolution for maximum axial resolution in three-dimensional aberration-corrected scanning transmission electron microscopy.

Authors:  Ranjan Ramachandra; Niels de Jonge
Journal:  Microsc Microanal       Date:  2011-12-08       Impact factor: 4.127

5.  The three-dimensional point spread function of aberration-corrected scanning transmission electron microscopy.

Authors:  Andrew R Lupini; Niels de Jonge
Journal:  Microsc Microanal       Date:  2011-08-31       Impact factor: 4.127

6.  Direct imaging of single metal atoms and clusters in the pores of dealuminated HY zeolite.

Authors:  Volkan Ortalan; Alper Uzun; Bruce C Gates; Nigel D Browning
Journal:  Nat Nanotechnol       Date:  2010-05-23       Impact factor: 39.213

7.  Three-dimensional scanning transmission electron microscopy of biological specimens.

Authors:  Niels de Jonge; Rachid Sougrat; Brian M Northan; Stephen J Pennycook
Journal:  Microsc Microanal       Date:  2010-02       Impact factor: 4.127

8.  Imaging the distribution of individual platinum-based anticancer drug molecules attached to single-wall carbon nanotubes.

Authors:  Ashwin A Bhirde; Alioscka A Sousa; Vyomesh Patel; Afrouz A Azari; J Silvio Gutkind; Richard D Leapman; James F Rusling
Journal:  Nanomedicine (Lond)       Date:  2009-10       Impact factor: 5.307

9.  Determination of atomic vacancies in InAs/GaSb strained-layer superlattices by atomic strain.

Authors:  Honggyu Kim; Yifei Meng; Ji-Hwan Kwon; Jean-Luc Rouviére; Jian Min Zuo
Journal:  IUCrJ       Date:  2018-01-01       Impact factor: 4.769

10.  In-line three-dimensional holography of nanocrystalline objects at atomic resolution.

Authors:  F-R Chen; D Van Dyck; C Kisielowski
Journal:  Nat Commun       Date:  2016-02-18       Impact factor: 14.919

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