Literature DB >> 16486989

Democratic particle motion for metabasin transitions in simple glass formers.

G A Appignanesi1, J A Rodríguez Fris, R A Montani, W Kob.   

Abstract

We use molecular dynamics computer simulations to investigate the local motion of the particles in a supercooled binary liquid. Using the concept of the distance matrix, we find that the alpha relaxation corresponds to a small number of crossings from one metabasin to a neighboring one. Each crossing is very rapid and involves the collective motion of O(40) particles that form a relatively compact cluster, whereas stringlike motions seem not to be relevant for these transitions. These compact clusters are thus potential candidates for the cooperatively rearranging regions proposed a long time ago by Adam and Gibbs.

Year:  2006        PMID: 16486989     DOI: 10.1103/PhysRevLett.96.057801

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  9 in total

1.  Correlation between dynamical heterogeneities, structure and potential-energy distribution in a 2D amorphous solid.

Authors:  S Mazoyer; F Ebert; G Maret; P Keim
Journal:  Eur Phys J E Soft Matter       Date:  2011-09-26       Impact factor: 1.890

2.  On the potential energy landscape of supercooled liquids and glasses.

Authors:  D Rodney; T Schrøder
Journal:  Eur Phys J E Soft Matter       Date:  2011-09-26       Impact factor: 1.890

3.  Structural and dynamical aspects of water in contact with a hydrophobic surface.

Authors:  D C Malaspina; E P Schulz; L M Alarcón; M A Frechero; G A Appignanesi
Journal:  Eur Phys J E Soft Matter       Date:  2010-05-22       Impact factor: 1.890

4.  Protein packing defects "heat up" interfacial water.

Authors:  María Belén Sierra; Sebastián R Accordino; J Ariel Rodriguez-Fris; Marcela A Morini; Gustavo A Appignanesi; Ariel Fernández Stigliano
Journal:  Eur Phys J E Soft Matter       Date:  2013-06-25       Impact factor: 1.890

5.  Evidence of a two-state picture for supercooled water and its connections with glassy dynamics.

Authors:  G A Appignanesi; J A Rodriguez Fris; F Sciortino
Journal:  Eur Phys J E Soft Matter       Date:  2009-07-16       Impact factor: 1.890

6.  Structure and dynamics of high- and low-density water molecules in the liquid and supercooled regimes.

Authors:  Joan Manuel Montes de Oca; J Ariel Rodriguez Fris; Sebastián R Accordino; David C Malaspina; Gustavo A Appignanesi
Journal:  Eur Phys J E Soft Matter       Date:  2016-12-15       Impact factor: 1.890

7.  Potential energy landscape activations governing plastic flows in glass rheology.

Authors:  Penghui Cao; Michael P Short; Sidney Yip
Journal:  Proc Natl Acad Sci U S A       Date:  2019-09-04       Impact factor: 11.205

8.  Quantitative investigation of the two-state picture for water in the normal liquid and the supercooled regime.

Authors:  S R Accordino; J A Rodriguez Fris; F Sciortino; G A Appignanesi
Journal:  Eur Phys J E Soft Matter       Date:  2011-05-16       Impact factor: 1.890

9.  Dynamic phase coexistence in glass-forming liquids.

Authors:  Raffaele Pastore; Antonio Coniglio; Massimo Pica Ciamarra
Journal:  Sci Rep       Date:  2015-07-09       Impact factor: 4.379

  9 in total

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