Literature DB >> 14683361

Internal laser-induced dipole force at work in C60 molecule.

V R Bhardwaj1, P B Corkum, D M Rayner.   

Abstract

We show how the many electron response of a complex molecule to an intense laser field can be incorporated with the single active electron picture. This enables us to introduce an "over-the-barrier" model for Cz+60 ionization, valid for long wavelength light. Using infrared radiation, we confirm the model and also produce stable, highly charged C60 reaching C12+60, the highest charge state ever observed. At high intensities and high charge states the internal laser-induced dipole force and rapid charging lead to stress on the molecule. The interplay between the forces provides control and suggest strategies for reaching even higher charge states.

Entities:  

Year:  2003        PMID: 14683361     DOI: 10.1103/PhysRevLett.91.203004

Source DB:  PubMed          Journal:  Phys Rev Lett        ISSN: 0031-9007            Impact factor:   9.161


  3 in total

1.  Cage connectivity and frontier π orbitals govern the relative stability of charged fullerene isomers.

Authors:  Yang Wang; Sergio Díaz-Tendero; Manuel Alcamí; Fernando Martín
Journal:  Nat Chem       Date:  2015-10-19       Impact factor: 24.427

2.  Laser induced C(60) cage opening studied by semiclassical dynamics simulation.

Authors:  Hong Tang; Hongjian Li; Yusheng Dou
Journal:  Int J Mol Sci       Date:  2011-01-13       Impact factor: 5.923

3.  The Role of Super-Atom Molecular Orbitals in Doped Fullerenes in a Femtosecond Intense Laser Field.

Authors:  Hui Xiong; Benoit Mignolet; Li Fang; Timur Osipov; Thomas J A Wolf; Emily Sistrunk; Markus Gühr; Francoise Remacle; Nora Berrah
Journal:  Sci Rep       Date:  2017-03-09       Impact factor: 4.379

  3 in total

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