On the use of LiF:Mg,Ti thermoluminescence dosemeters in space--a critical review.

The use of LiF:Mg,Ti thermoluminescence dosemeters (TLDs) in space radiation fields is reviewed. It is demonstrated in the context of modified track structure theory and microdosimetric track structure theory that there is no unique correlation between the relative thermoluminescence (TL) efficiency of heavy charged particles, neutrons of all energies and linear energy transfer (LET). Many experimental measurements dating back more than two decades also demonstrate the multivalued, non-universal, relationship between relative TL efficiency and LET. It is further demonstrated that the relative intensities of the dosimetric peaks and especially the high-temperature structure are dependent on a large number of variables, some controllable, some not. It is concluded that TL techniques employing the concept of LET (e.g. measurement of total dose, the high-temperature ratio (HTR) methods and other combinations of the relative TL efficiency of the various peaks used to estimate average Q or simulate Q-LET relationships) should be regarded as lacking a sound theoretical basis, highly prone to error and, as well, lack of reproducibility/universality due to the absence of a standardised experimental protocol essential to reliable experimental methodology.