Literature DB >> 14500975

Ultrafast hydrogen-bond dynamics in the infrared spectroscopy of water.

C J Fecko1, J D Eaves, J J Loparo, A Tokmakoff, P L Geissler.   

Abstract

We investigated rearrangements of the hydrogen-bond network in water by measuring fluctuations in the OH-stretching frequency of HOD in liquid D2O with femtosecond infrared spectroscopy. Using simulations of an atomistic model of water, we relate these frequency fluctuations to intermolecular dynamics. The model reveals that OH frequency shifts arise from changes in the molecular electric field that acts on the proton. At short times, vibrational dephasing reflects an underdamped oscillation of the hydrogen bond with a period of 170 femtoseconds. At longer times, vibrational correlations decay on a 1.2-picosecond time scale because of collective structural reorganizations.

Entities:  

Year:  2003        PMID： 14500975     DOI： 10.1126/science.1087251

Source DB:  PubMed          Journal:  Science        ISSN： 0036-8075            Impact factor:   47.728


  91 in total

Review 1.  Vibrational Spectroscopic Map, Vibrational Spectroscopy, and Intermolecular Interaction.

Authors:  Carlos R Baiz; Bartosz Błasiak; Jens Bredenbeck; Minhaeng Cho; Jun-Ho Choi; Steven A Corcelli; Arend G Dijkstra; Chi-Jui Feng; Sean Garrett-Roe; Nien-Hui Ge; Magnus W D Hanson-Heine; Jonathan D Hirst; Thomas L C Jansen; Kijeong Kwac; Kevin J Kubarych; Casey H Londergan; Hiroaki Maekawa; Mike Reppert; Shinji Saito; Santanu Roy; James L Skinner; Gerhard Stock; John E Straub; Megan C Thielges; Keisuke Tominaga; Andrei Tokmakoff; Hajime Torii; Lu Wang; Lauren J Webb; Martin T Zanni
Journal:  Chem Rev       Date:  2020-06-29       Impact factor: 60.622

2.  A two-dimensional infrared study of localization, structure, and dynamics of a dipeptide in membrane environment.

Authors:  V Volkov; P Hamm
Journal:  Biophys J       Date:  2004-09-17       Impact factor: 4.033

3.  Real-time mapping of electronic structure with single-shot two-dimensional electronic spectroscopy.

Authors:  Elad Harel; Andrew F Fidler; Gregory S Engel
Journal:  Proc Natl Acad Sci U S A       Date:  2010-09-01       Impact factor: 11.205

4.  Redrawing the Ramachandran plot after inclusion of hydrogen-bonding constraints.

Authors:  Lauren L Porter; George D Rose
Journal:  Proc Natl Acad Sci U S A       Date:  2010-12-08       Impact factor: 11.205

5.  The nano-structural inhomogeneity of dynamic hydrogen bond network of TIP4P/2005 water.

Authors:  Vladimir Belosludov; Kirill Gets; Ravil Zhdanov; Valery Malinovsky; Yulia Bozhko; Rodion Belosludov; Nikolay Surovtsev; Oleg Subbotin; Yoshiyuki Kawazoe
Journal:  Sci Rep       Date:  2020-04-30       Impact factor: 4.379

6.  Spectral diffusion in a fluctuating charge model of water.

Authors:  S A Corcelli; C P Lawrence; J B Asbury; T Steinel; M D Fayer; J L Skinner
Journal:  J Chem Phys       Date:  2004-11-08       Impact factor: 3.488

7.  Dynamics of confined water molecules.

Authors:  J J Gilijamse; A J Lock; H J Bakker
Journal:  Proc Natl Acad Sci U S A       Date:  2005-02-18       Impact factor: 11.205

8.  Quantum corrections in vibrational and electronic condensed phase spectroscopy: line shapes and echoes.

Authors:  C P Lawrence; J L Skinner
Journal:  Proc Natl Acad Sci U S A       Date:  2005-04-22       Impact factor: 11.205

9.  The dynamics of peptide-water interactions in dialanine: An ultrafast amide I 2D IR and computational spectroscopy study.

Authors:  Chi-Jui Feng; Andrei Tokmakoff
Journal:  J Chem Phys       Date:  2017-08-28       Impact factor: 3.488

10.  Hydrogen bonding and Raman, IR, and 2D-IR spectroscopy of dilute HOD in liquid D2O.

Authors:  B Auer; R Kumar; J R Schmidt; J L Skinner
Journal:  Proc Natl Acad Sci U S A       Date:  2007-06-18       Impact factor: 11.205
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