Attosecond active synchronization of passively mode-locked lasers by balanced cross correlation.

A balanced cross correlator, the optical equivalent of a balanced microwave phase detector, is demonstrated. Its use in synchronizing an octave-spanning Ti:sapphire laser and a 30-fs Cr:forsterite laser yields 300-attosecond timing jitter measured from 10 mHz to 2.3 MHz. The spectral overlap between the two lasers is strong enough to permit direct detection of the difference in carrier-envelope offset frequency between the two lasers.